Surface enhanced vibrational spectroscopic evidence for an alternative DNA-independent redox activation of endonuclease III

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Abstract

Surface enhanced vibrational spectro-electrochemistry of endonuclease III provides direct evidence that the [4Fe-4S] cluster is responsible for the enzyme redox activity, and that this process is not exclusively DNA-mediated, as currently proposed. We report the first surface enhanced resonance Raman spectrum of a [4Fe-4S]2+ cluster containing enzyme.

Original languageEnglish
Pages (from-to)3255-3257
Number of pages3
JournalChemical Communications
Volume51
Issue number15
DOIs
Publication statusPublished - 21 Feb 2015

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