TY - JOUR
T1 - Solution Combustion Synthesis
T2 - Towards a Sustainable Approach for Metal Oxides
AU - Carlos, Emanuel
AU - Martins, Rodrigo
AU - Fortunato, Elvira
AU - Branquinho, Rita
N1 - info:eu-repo/grantAgreement/EC/H2020/685758/EU#
info:eu-repo/grantAgreement/EC/H2020/817161/EU#
info:eu-repo/grantAgreement/EC/H2020/787410/EU#
This work is funded by National Funds through FCT-Portuguese Foundation for Science and Technology, Reference UID/CTM/50025/2019 and FCT/MCTES.
E.C, acknowledges FCT/MCTES for a doctoral grant (Grant SFRH/BD/116047/2016) and IDS-FunMat-INNO project FPA2016/EIT/EIT RawMaterials Grant Agreement 15015.
PY - 2020/7/27
Y1 - 2020/7/27
N2 - Solution combustion synthesis (SCS) has been widely used to produce simple and complex oxides with a desired morphology (size and shape). SCS is valuable due to low cost, simplicity and energy efficient synthesis. To guarantee the best molecular-level mixing of reactants in an aqueous or solvent-based solution some parameters need to be controlled, such as fuel type, metal cations precursors, stoichiometry ratio (φ), pH effect, atmosphere and initiation type. These determine the final properties of the oxide materials, providing the potential to reach different morphologies, which are essential for their final applications. This Review article focuses on the crucial parameters in SCS and how these affect the overall materials properties from nanostructures to thin films. To finalize, special attention is given to the application of SCS to form metal oxide thin films at low temperature and their application in thin film transistors (TFTs).
AB - Solution combustion synthesis (SCS) has been widely used to produce simple and complex oxides with a desired morphology (size and shape). SCS is valuable due to low cost, simplicity and energy efficient synthesis. To guarantee the best molecular-level mixing of reactants in an aqueous or solvent-based solution some parameters need to be controlled, such as fuel type, metal cations precursors, stoichiometry ratio (φ), pH effect, atmosphere and initiation type. These determine the final properties of the oxide materials, providing the potential to reach different morphologies, which are essential for their final applications. This Review article focuses on the crucial parameters in SCS and how these affect the overall materials properties from nanostructures to thin films. To finalize, special attention is given to the application of SCS to form metal oxide thin films at low temperature and their application in thin film transistors (TFTs).
KW - fuel
KW - metal oxides
KW - nanostructures
KW - solution combustion synthesis
KW - thin film transistors
U2 - 10.1002/chem.202000678
DO - 10.1002/chem.202000678
M3 - Review article
C2 - 32134133
SN - 0947-6539
VL - 26
SP - 9099
EP - 9125
JO - Chemistry - A European Journal
JF - Chemistry - A European Journal
IS - 42
ER -