TY - JOUR
T1 - Printed Zinc Tin Oxide Memristors for Reservoir Computing
AU - Azevedo Martins, Raquel
AU - Silva, Carlos
AU - Deuermeier, Jonas
AU - Milano, Gianluca
AU - Rosero-Realpe, Mateo
AU - Parreira, Carolina
AU - Fortunato, Elvira
AU - Martins, Rodrigo
AU - Kiazadeh, Asal
AU - Carlos, Emanuel
N1 - info:eu-repo/grantAgreement/FCT/Concurso para Atribuição do Estatuto e Financiamento de Laboratórios Associados (LA)/LA%2FP%2F0037%2F2020/PT#
info:eu-repo/grantAgreement/FCT/Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017%2F2018) - Financiamento Programático/UIDP%2F50025%2F2020/PT#
info:eu-repo/grantAgreement/FCT/Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017%2F2018) - Financiamento Base/UIDB%2F50025%2F2020/PT#
info:eu-repo/grantAgreement/FCT/OE/2022.13773.BD/PT#
info:eu-repo/grantAgreement/FCT//2021.07840.BD/PT#
info:eu-repo/grantAgreement/FCT/CEEC IND4ed/2021.03825.CEECIND%2FCP1657%2FCT0015/PT#
info:eu-repo/grantAgreement/FCT/CEEC IND4ed/2021.03386.CEECIND%2FCP1657%2FCT0002/PT#
info:eu-repo/grantAgreement/FCT/3599-PPCDT/2022.08132.PTDC/PT#
info:eu-repo/grantAgreement/FCT/Projetos de IC&DT Portugal Índia/DRI%2FIndia%2F0430%2F2020/PT#
Funding Information:
This work was financed by national funds from FCT-Fundação para a Ciência e a Tecnologia, I.P., in the scope of the projects LA/P/0037/2020, UIDP/50025/2020, and UIDB/50025/2020 of the Associate Laboratory Institute of Nanostructures, Nanomodelling and Nanofabrication–i3N. R.A.M. and C.S. thank the Fundação para a Ciência e Tecnologia (FCT) for financial support under the Ph.D. grants (2022.13773.BD and 2021.07840.BD). E.C., A.K., and J.D. acknowledge funding received from FCT via 2021.03825.CEECIND, 2021.03386.CEECIND, and CEECINST/00102/2018, respectively. The authors acknowledge the FCT for funding received with project OPERA via 2022.08132.PTDC and project VOCMemsense via DRI/India/0430/2020. The authors further acknowledge the TERRAMETA project no.10109710. This work also received funding from the HORIZONEIC-2023-PATHFINDERCHALLENGES-01 program, grant agreement
no. 101161114 (ELEGANCE). G.M. acknowledges the support of the European Research Council (ERC) under the European Union’s ERC Staring grant (ERC-2024-STG) agreement “MEMBRAIN” no. 101 160 604.
Publisher Copyright:
© 2025 The Author(s). Advanced Intelligent Systems published by Wiley-VCH GmbH.
PY - 2025/8/3
Y1 - 2025/8/3
N2 - In this work, fully patterned zinc tin oxide (ZTO) memristors are introduced using inkjet printing. By targeting a scalable, solution-based fabrication approach, highly stable devices with excellent reproducibility and minimal variability are achieved, using ZTO as the active layer, silver (Ag) as the top electrode, and molybdenum as the bottom electrode. The use of sustainable materials like ZTO enhances scalability and environmental compatibility, paving the way for next-generation, low-power neuromorphic computing. The devices successfully fulfill the fundamental criteria for in materia implementation of physical reservoir computing (PRC), including nonlinearity and fading memory property. The devices are successfully trained for classification tasks with MNIST handwritten dataset, achieving 89.4% accuracy and 86.5% by processing 4-bit and 5-bit input temporal sequences. The integration of printed memristors into hardware-based PRC architecture simplifies training complexity, making them particularly advantageous for energy-efficient, wearable AI systems.
AB - In this work, fully patterned zinc tin oxide (ZTO) memristors are introduced using inkjet printing. By targeting a scalable, solution-based fabrication approach, highly stable devices with excellent reproducibility and minimal variability are achieved, using ZTO as the active layer, silver (Ag) as the top electrode, and molybdenum as the bottom electrode. The use of sustainable materials like ZTO enhances scalability and environmental compatibility, paving the way for next-generation, low-power neuromorphic computing. The devices successfully fulfill the fundamental criteria for in materia implementation of physical reservoir computing (PRC), including nonlinearity and fading memory property. The devices are successfully trained for classification tasks with MNIST handwritten dataset, achieving 89.4% accuracy and 86.5% by processing 4-bit and 5-bit input temporal sequences. The integration of printed memristors into hardware-based PRC architecture simplifies training complexity, making them particularly advantageous for energy-efficient, wearable AI systems.
KW - fully patterned
KW - memristor
KW - physical reservoir computing
KW - printed memristors
KW - solution-based
KW - ZTO
UR - https://www.scopus.com/pages/publications/105012218494
U2 - 10.1002/aisy.202500450
DO - 10.1002/aisy.202500450
M3 - Article
AN - SCOPUS:105012218494
SN - 2640-4567
JO - Advanced Intelligent Systems
JF - Advanced Intelligent Systems
M1 - 2500450
ER -