Photochemical modification of a diamond surface using a pulsed UV laser as the energy source

Mariana Silva, Nádia E. Santos, Mariana Pinto, Samuel Guieu, Ricardo Oliveira, Flávio Figueira, Filipe A.Almeida Paz, Miguel Neto, Luis Rino, Jonas Deuermeier, Milan Maradiya, Michael Liehr, Joana C. Mendes, Susana S. Braga

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Abstract

The use of an excimer benchtop pulsed UV laser as the energy source for the photochemical modification of the surface of diamond films is reported. Boron-doped nanocrystalline diamond (NCD) films were deposited on Si wafers via plasma-enhanced chemical vapour deposition (PECVD). The as-deposited films were characterised by scanning electron microscopy (SEM), Raman spectroscopy, and X-ray diffraction (XRD). Following characterisation, the surfaces of the films were subjected to a photochemical reaction with 2,2,2-trifluoroethyl undec-10-enoate using two different sources of radiation: a benchtop UV lamp (254 nm) and a KrF excimer pulsed UV laser (248 nm). The photochemically treated films were characterised by contact angle measurements and X-ray photoelectric spectroscopy (XPS) using non-treated films as a control. The use of a pulsed UV laser source was shown to reduce the photochemical reaction time from several hours to a few minutes.

Original languageEnglish
Article number111314
JournalDiamond and Related Materials
Volume147
DOIs
Publication statusPublished - Aug 2024

Keywords

  • Biosensor
  • Diamond
  • Photochemical reactions
  • Surface chemistry
  • UV laser

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